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Visible-Light-Promoted Oxo-Sulfonylation of Ynamides with Sulfonic Acids
A visible-light-promoted oxo-sulfonylation of ynamides with sulfonic acids is reported, giving rise to a collection of functionalized alpha-sulfonylated amides in a straightforward manner. The reaction proceeds sequentially through a cascade of electrophilic addition and photoinduced sulfonyl radical-sustained skeleton rearrangement. The high atom economy, mild reaction conditions, and wide substrate scope comprised the merits of this synthetic transformation.
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Reference：
Quinuclidine – Wikipedia,
Quinuclidine | C7H475N | ChemSpider